Thickened battery electrodes pave the way for fast-charging EVs

Researchers at the University of Texas at Austin have fabricated a new type of electrode for lithium-ion batteries that could facilitate greater power and faster charging for electric vehicles. This was achieved by creating thicker electrodes — the positively and negatively charged parts of the battery that deliver power to a device — using magnets to create a unique alignment that sidesteps the common problems associated with sizing up these components. The result is an electrode that could potentially facilitate twice the range on a single charge for an electric vehicle, compared with a battery using an existing commercial electrode.

Guihua Yu, a professor in UT Austin’s Walker Department of Mechanical Engineering and Texas Materials Institute, said that two-dimensional materials are thought to be a promising candidate for high-rate energy storage applications because they only need to be several nanometres thick for rapid charge transport. “However, for thick-electrode-design-based next-generation, high-energy batteries, the restacking of nanosheets as building blocks can cause significant bottlenecks in charge transport, leading to difficulty in achieving both high energy and fast charging,” Yu said.

The key to the discovery, published in the Proceedings of the National Academy of Sciences, uses thin two-dimensional materials as the building blocks of the electrode, stacking them to create thickness and then using a magnetic field to manipulate their orientations. The research team used commercially available magnets during fabrication to arrange the two-dimensional materials in a vertical alignment, creating a fast lane for ions to travel through the electrode. Typically, thicker electrodes force the ions to travel longer distances to move through the battery, which leads to slower charging time. The typical horizontal alignment of the layers of material that make up the electrode force the ions to snake back and forth.

“Our electrode shows superior electrochemical performance partially due to the high mechanical strength, high electrical conductivity and facilitated lithium-ion transport thanks to the unique architecture we designed,” said Zhengyu Ju, a graduate student who is leading this project.

In addition to comparing their electrode with a commercial electrode, researchers also fabricated a horizontally arranged electrode using the same materials for experimental control purposes. Through this, they recharged the vertical thick electrode to 50% energy level in 30 minutes, compared with two hours and 30 minutes with the horizontal electrode. Although the researchers looked at just a single type of battery electrode in this research, their goal is to generalise their methodology of vertically organised electrode layers to apply it to different types of electrodes using other materials. This could help the technique become more widely adopted in industry, so it could enable future fast-charging yet high-energy batteries that power electric vehicles.

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